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OpenQDC: Open Quantum Data Commons

2024-11-29 · Cristian Gabellini, Nikhil Shenoy, Stephan Thaler, Semih Canturk, Daniel McNeela, Dominique Beaini, Michael Bronstein, Prudencio Tossou

Machine Learning Interatomic Potentials (MLIPs) are a highly promising alternative to force-fields for molecular dynamics (MD) simulations, offering precise and rapid energy and force calculations. However, Quantum-Mechanical (QM) datasets, crucial for MLIPs, are fragmented across various repositories, hindering accessibility and model development. We introduce the openQDC package, consolidating 37 QM datasets from over 250 quantum methods and 400 million geometries into a single, accessible resource. These datasets are meticulously preprocessed, and standardized for MLIP training, covering a wide range of chemical elements and interactions relevant in organic chemistry. OpenQDC includes tools for normalization and integration, easily accessible via Python. Experiments with well-known architectures like SchNet, TorchMD-Net, and DimeNet reveal challenges for those architectures and constitute a leaderboard to accelerate benchmarking and guide novel algorithms development. Continuously adding datasets to OpenQDC will democratize QM dataset access, foster more collaboration and innovation, enhance MLIP development, and support their adoption in the MD field.

📄 PDF Abstract BibTeX arXiv:2411.19629

Code (1)

valence-labs/OpenQDC 공식 구현

Tasks

Benchmarking

Methods 이 논문이 사용한 방법론

Shifted Softplus Shifted Softplus is an activation function ${\rm ssp}(x) = \ln( 0.5 e^{x} + 0.5 )$, which SchNet employs as non-linearity…
SchNet SchNet is an end-to-end deep neural network architecture based on continuous-filter convolutions. It follows the deep tensor neural network framework, i.e. atom-wise…

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