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SE3Set: Harnessing equivariant hypergraph neural networks for molecular representation learning

2024-05-26 · Hongfei Wu, Lijun Wu, Guoqing Liu, Zhirong Liu, Bin Shao, Zun Wang

In this paper, we develop SE3Set, an SE(3) equivariant hypergraph neural network architecture tailored for advanced molecular representation learning. Hypergraphs are not merely an extension of traditional graphs; they are pivotal for modeling high-order relationships, a capability that conventional equivariant graph-based methods lack due to their inherent limitations in representing intricate many-body interactions. To achieve this, we first construct hypergraphs via proposing a new fragmentation method that considers both chemical and three-dimensional spatial information of molecular system. We then design SE3Set, which incorporates equivariance into the hypergragh neural network. This ensures that the learned molecular representations are invariant to spatial transformations, thereby providing robustness essential for accurate prediction of molecular properties. SE3Set has shown performance on par with state-of-the-art (SOTA) models for small molecule datasets like QM9 and MD17. It excels on the MD22 dataset, achieving a notable improvement of approximately 20% in accuracy across all molecules, which highlights the prevalence of complex many-body interactions in larger molecules. This exceptional performance of SE3Set across diverse molecular structures underscores its transformative potential in computational chemistry, offering a route to more accurate and physically nuanced modeling.

📄 PDF Abstract BibTeX arXiv:2405.16511

Code (1)

Navantock/SE3Set 공식 구현 pytorch

Tasks

Computational chemistrymolecular representationRepresentation Learning

Methods 이 논문이 사용한 방법론

Fragmentation Given a pattern $P,$ that is more complicated than the patterns, we fragment $P$ into simpler patterns such that their exact count is known. In the subgraph GNN proposed earlier,…

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