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Perfecting Liquid-State Theories with Machine Intelligence

2023-11-09 · Jianzhong Wu, Mengyang Gu

Recent years have seen a significant increase in the use of machine intelligence for predicting electronic structure, molecular force fields, and the physicochemical properties of various condensed systems. However, substantial challenges remain in developing a comprehensive framework capable of handling a wide range of atomic compositions and thermodynamic conditions. This perspective discusses potential future developments in liquid-state theories leveraging on recent advancements of functional machine learning. By harnessing the strengths of theoretical analysis and machine learning techniques including surrogate models, dimension reduction and uncertainty quantification, we envision that liquid-state theories will gain significant improvements in accuracy, scalability and computational efficiency, enabling their broader applications across diverse materials and chemical systems.

📄 PDF Abstract BibTeX arXiv:2311.05167

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Computational EfficiencyDimensionality ReductionUncertainty Quantification

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